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posted by martyb on Wednesday August 28 2019, @06:00AM   Printer-friendly
from the getting-H2O2-out-of-thin-air^W-water dept.

Water is everywhere on Earth, but maybe that just gives it more space to hide its secrets. Its latest surprise, Stanford researchers report Aug. 26 in Proceedings of the National Academy of Sciences, is that microscopic droplets of water spontaneously produce hydrogen peroxide.

The discovery could pave the way for greener ways to produce the molecule, a common bleaching agent and disinfectant, said Richard Zare, the Marguerite Blake Wilbur Professor in Natural Science and a professor of chemistry in the Stanford School of Humanities and Sciences.

"Water is one of the most commonly found materials, and it's been studied for years and years and you would think that there was nothing more to learn about this molecule. But here's yet another surprise," said Zare, who is also a member of Stanford Bio-X.

The discovery was made serendipitously while Zare and his lab were studying a new, more efficient way to create gold nanostructures in tiny water droplets known as microdroplets. To make those structures, the team added an additional molecule called a reducing agent. As a control test, Zare suggested seeing if they could create gold nanostructures without the reducing agent. Theoretically that should have been impossible, but it worked anyway—hinting at an as yet undiscovered feature of microdroplet chemistry.

https://phys.org/news/2019-08-chemists-microdroplets-spontaneously-hydrogen-peroxide.html

First astrology and now homeopathy are starting to make sense after all.

Jae Kyoo Lee el al., "Spontaneous generation of hydrogen peroxide from aqueous microdroplets", PNAS (2019). www.pnas.org/cgi/doi/10.1073/pnas.1911883116


Original Submission

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Study Corroborates the Influence of Planetary Tidal Forces on Solar Activity 31 comments

One of the big questions in solar physics is why the sun's activity follows a regular cycle of 11 years. Researchers from the Helmholtz-Zentrum Dresden-Rossendorf (HZDR), an independent German research institute, now present new findings, indicating that the tidal forces of Venus, Earth and Jupiter influence the solar magnetic field, thus governing the solar cycle.

[...] To accomplish this result, the scientists systematically compared historical observations of solar activity from the last thousand years with planetary constellations, statistically proving that the two phenomena are linked. "There is an astonishingly high level of concordance: what we see is complete parallelism with the planets over the course of 90 cycles," said Frank Stefani, lead author of the study. "Everything points to a clocked process."

[...] Besides influencing the 11-year cycle, planetary tidal forces may also have other effects on the sun. For example, it is also conceivable that they change the stratification of the plasma in the transition region between the interior radiative zone and the outer convection zone of the sun (the tachocline) in such a way that the magnetic flux can be conducted more easily. Under those conditions, the magnitude of activity cycles could also be changed, as was once the case with the Maunder Minimum, when there was a strong decline in solar activity for a longer phase.

https://phys.org/news/2019-05-corroborates-planetary-tidal-solar.html


Original Submission

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  • (Score: 0) by Anonymous Coward on Wednesday August 28 2019, @06:02AM

    by Anonymous Coward on Wednesday August 28 2019, @06:02AM (#886663)

    N/A

  • (Score: 2) by c0lo on Wednesday August 28 2019, @06:38AM (9 children)

    by c0lo (156) Subscriber Badge on Wednesday August 28 2019, @06:38AM (#886674) Journal

    What the fucking fuck? Hydrogen peroxide is an oxidant, not a reducing agent!

    --
    https://www.youtube.com/@ProfSteveKeen https://soylentnews.org/~MichaelDavidCrawford
    • (Score: 2) by coolgopher on Wednesday August 28 2019, @06:58AM (1 child)

      by coolgopher (1157) on Wednesday August 28 2019, @06:58AM (#886679)

      The team eventually traced those results to the presence of a molecule called hydroxyl—a single hydrogen atom paired with an oxygen atom — that can also act as a reducing agent.

      You may untwist your knickers now.

      • (Score: 2) by c0lo on Wednesday August 28 2019, @07:06AM

        by c0lo (156) Subscriber Badge on Wednesday August 28 2019, @07:06AM (#886683) Journal

        You may untwist your knickers now.

        Not completely yet. No energy considerations, not confirmed as 'it is the size that matter' (they did it by water atomization only, how about they do it in fog droplets?), etc.

        --
        https://www.youtube.com/@ProfSteveKeen https://soylentnews.org/~MichaelDavidCrawford
    • (Score: 4, Informative) by c0lo on Wednesday August 28 2019, @07:00AM (5 children)

      by c0lo (156) Subscriber Badge on Wednesday August 28 2019, @07:00AM (#886680) Journal

      TFAbstract [pnas.org]

      We show H2O2 is spontaneously produced from pure water by atomizing bulk water into microdroplets (1 μm to 20 µm in diameter). Production of H2O2, as assayed by H2O2-sensitve fluorescence dye peroxyfluor-1, increased with decreasing microdroplet size. Cleavage of 4-carboxyphenylboronic acid and conversion of phenylboronic acid to phenols in microdroplets further confirmed the generation of H2O2. The generated H2O2 concentration was ∼30 µM (∼1 part per million) as determined by titration with potassium titanium oxalate. Changing the spray gas to O2 or bubbling O2 decreased the yield of H2O2 in microdroplets, indicating that pure water microdroplets directly generate H2O2 without help from O2 either in air surrounding the droplet or dissolved in water. We consider various possible mechanisms for H2O2 formation and report a number of different experiments exploring this issue. We suggest that hydroxyl radical (OH) recombination is the most likely source, in which OH is generated by loss of an electron from OH− at or near the surface of the water microdroplet. This catalyst-free and voltage-free H2O2 production method provides innovative opportunities for green production of hydrogen peroxide.

      Essentially, they are saying that, in small water droplets, free OH- radicals (which are reducing agents) are observable at higher call concentration than in bulk water, that those radicals lose easier their electron and recombine in pairs to form hydrogen peroxide.

      I'm curious if someone manages to reproduce the experiment. 'Cause one of the consequences would be that splitting water and obtaining hydrogen is possible by atomizing water. I doubt it happens simply because of the size of water droplets, as fog/clouds have sizes in the range reported by TFA [uwyo.edu]. No matter the low concentration, over.hundred of millions of years of raining, a significant proportion of water would be lost by the loss of hydrogen.

      --
      https://www.youtube.com/@ProfSteveKeen https://soylentnews.org/~MichaelDavidCrawford
      • (Score: 1, Interesting) by Anonymous Coward on Wednesday August 28 2019, @07:56AM (1 child)

        by Anonymous Coward on Wednesday August 28 2019, @07:56AM (#886693)

        'Cause one of the consequences would be that splitting water and obtaining hydrogen is possible by atomizing water.

        The following is in equilibruim normally, which defines the pH of water (negative logarithm of the H3O+ concentration).

        H2O + H2O = H3O+ + HO-

        So, the interesting part is going from HO- to H2O2 without a catalyst and preventing reacting back to water with the acid.

        • (Score: 3, Interesting) by c0lo on Wednesday August 28 2019, @08:59AM

          by c0lo (156) Subscriber Badge on Wednesday August 28 2019, @08:59AM (#886709) Journal

          There something interesting in the phys.org FA too:

          Additional tests confirmed that water microdroplets spontaneously form hydrogen peroxide, that smaller microdroplets produced higher concentrations of the molecule, and that hydrogen peroxide was not lost when the microdroplets recombined into bulk water.

          Which suggest that somehow the system evolved in a state of higher energy. The only explanation I can imagine: a higher energy metastable state that was reached by the atomization process; perhaps a charge separation between droplets and the gas used in atomization too.

          --
          https://www.youtube.com/@ProfSteveKeen https://soylentnews.org/~MichaelDavidCrawford
      • (Score: 0) by Anonymous Coward on Wednesday August 28 2019, @10:35AM (2 children)

        by Anonymous Coward on Wednesday August 28 2019, @10:35AM (#886724)

        Changing the spray gas to O2 or bubbling O2 decreased the yield of H2O2 in microdroplets, indicating that pure water microdroplets directly generate H2O2 without help from O2 either in air surrounding the droplet or dissolved in water.

        But did they change the spray gas to pure N2? For "strange stuff" like this wouldn't testing with pure nitrogen be the correct way to prove that the H2O2 is generated without help from O2 in air?

        Being thorough and eliminating most of the O2 dissolved in the water is a bit harder but I don't think it's impossible.

        But I suppose this sort of stuff is for the next publication? The joys of "publish or perish" driven "science"... ;)

        • (Score: 3, Interesting) by All Your Lawn Are Belong To Us on Wednesday August 28 2019, @03:19PM (1 child)

          by All Your Lawn Are Belong To Us (6553) on Wednesday August 28 2019, @03:19PM (#886833) Journal

          Or..... genuine science. Where one person or group uses one's thinker as best as one can, one notices an anomaly, one comes up with a null hypothesis, one does one's best to eliminate confounding variables but in the end design the best experiment one can, have at the experiment, record the results, then test to see if the null hypothesis is sustained. And then most importantly: One places one's results in public view and invites both criticism and makes it possible for others to follow well enough to test themselves to confirm or deny what the truth is for themselves.

          If I get what they did - they always used a reagent to get their results, they removed that reagent and still got results, they came up with a how it might be possible and devised a test to confirm if H2O2 was being produced by something other than their reagent and it is. I may be reading that wrong, but there one is. The PNAS abstract quoted above says, "Water molecules are spontaneously oxidized to form hydrogen peroxide near the water−air interface of micron-sized water droplets. This process does not require any chemical reagent, catalyst, applied electric potential, or radiation. Only pure water in the form of microdroplets in air is necessary for the appearance of hydrogen peroxide." Although the phys.org article on phys.org says they were using strong electric fields in the vicinity and that could be the reason (which is different from an applied electrical potential... I suppose?????) Don't have time to determine if phys.org is summarizing it wrong or if there's a house of cards here or what.

          --
          This sig for rent.
          • (Score: 0) by Anonymous Coward on Wednesday August 28 2019, @03:26PM

            by Anonymous Coward on Wednesday August 28 2019, @03:26PM (#886838)

            one comes up with a null hypothesis

            Once you are coming up with a "null hypothesis" you are pretty much fucked. People doing science come up with "their hypothesis", not a "null hypothesis". Einstein (actually whoever was running those experiments) didn't check whether the apparent position of the stars moved exactly 0 degrees from expected during an eclipse. He checked whether they appeared to move the amount his theory predicted.

    • (Score: 1, Interesting) by Anonymous Coward on Wednesday August 28 2019, @02:08PM

      by Anonymous Coward on Wednesday August 28 2019, @02:08PM (#886789)

      Here. Explains it better than I could. [unl.edu]
      For the non-link clickers,

      When H2O2 serves as an oxidizing agent, the oxygen is reduced to H2O. When H2O2 serves as a reducing agent, the oxygen is oxidized to O2 and bubbles are noticed.

      It's role changes depending on the reagent.
      Replicated any number of places.
      But I agree that it is a weird property.

  • (Score: 2, Interesting) by Anonymous Coward on Wednesday August 28 2019, @01:34PM

    by Anonymous Coward on Wednesday August 28 2019, @01:34PM (#886771)

    Hahnemann found that undiluted doses caused reactions, sometimes dangerous ones, so specified that preparations be given at the lowest possible dose. He found that this reduced potency as well as side-effects, but formed the view that vigorous shaking and striking on an elastic surface – a process he termed Schütteln, translated as succussion – nullified this.[94] A common explanation for his settling on this process is said to be that he found preparations subjected to agitation in transit, such as in saddle bags or in a carriage, were more "potent".[62]:16 Hahnemann had a saddle-maker construct a special wooden striking board covered in leather on one side and stuffed with horsehair.[95]:31 Insoluble solids, such as granite, diamond, and platinum, are diluted by grinding them with lactose ("trituration").[62]:23

    The process of dilution and succussion is termed "dynamization" or "potentization" by homeopaths.[9][96] In industrial manufacture this may be done by machine.

    Serial dilution is achieved by taking an amount of the mixture and adding solvent, but the "Korsakovian" method may also be used, whereby the vessel in which the preparations are manufactured is emptied, refilled with solvent, and the volume of fluid adhering to the walls of the vessel is deemed sufficient for the new batch.

    https://en.wikipedia.org/wiki/Homeopathy#Preparation [wikipedia.org]

    They (the "real" homeopaths who actually follow the protocol) either use what sticks to the side of the vessel or skim the top after vigorous shaking. So it is not a random sample of the solution that gets passed from one dilution to the next.

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